Dynamical analysis of the effect of elliptically polarized laser pulses on molec

In this Letter, we study the molecular alignment and orientation driven by two elliptically polarized laser pulses. It is shown that the field-free molecular alignment can be achieved in a three-dimensional (3D) case, while the field-free molecular orientation is only along the x and y directions, and that the field-free alignment and orientation along different axes are related to the populations of the rotational states. It is demonstrated that changing the elliptic parameter is efficient for